The possible threat of radicalization among prison inmates has received widespread political and public attention in Europe. Several countries, including the Netherlands, seek to prevent prisoner radicalization by detaining violent extremist offenders together in segregated high-security facilities. However, it is unclear whether or not such policies are based on sound rationale. This study aims to conduct an in-depth evaluation of terrorism detention policy, based on extensive research among policy makers, prison staff, and prisoners in the Netherlands.